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A new catalyst-embedded hierarchical air electrode for high-performance Li-O-2 batteries

Cited 112 time in Web of Science Cited 115 time in Scopus
Authors
Lim, Hee-Dae; Song, Hyelynn; Gwon, Hyeokjo; Park, Kyu-Young; Kim, Jinsoo; Bae, Youngjoon; Kim, Hyungsub; Jung, Sung-Kyun; Kim, Taewoo; Kim, Yong Hyup; Lepro, Xavier; Ovalle-Robles, Raquel; Baughman, Ray H.; Kang, Kisuk
Issue Date
2013-12
Citation
Energy and Environmental Sciences, Vol.6 No.12, pp.3570-3575
Abstract
The Li-O-2 battery holds great promise as an ultra-high-energydensity device. However, its limited rechargeability and low energy efficiency remain key barriers to its practical application. Herein, we demonstrate that the ideal electrode morphology design combined with effective catalyst decoration can enhance the rechargeability of the Li-O-2 battery over 100 cycles with full discharge and charge. An aligned carbon structure with a hierarchical micro-nano-mesh ensures facile accessibility of reaction products and provides the optimal catalytic conditions for the Pt catalyst. The new electrode is highly reversible even at the extremely high current rate of 2 A g(-1). Moreover, we observed clearly distinct morphologies of discharge products when the catalyst is used. The effect of catalysts on the cycle stability is discussed.
ISSN
1754-5692
URI
http://hdl.handle.net/10371/165128
DOI
https://doi.org/10.1039/c3ee41910j
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College of Engineering/Engineering Practice School (공과대학/대학원)Dept. of Material Science and Engineering (재료공학부) Journal Papers (저널논문_재료공학부)
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