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Polarized Raman scattering of epitaxial PbTiO3 thin films with coexisting c- and a-domains

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Authors
Lee, Sun-Hwa; Jang, Hyun M.; Cho, Seong M.; Yi, Gyu-Chul
Issue Date
2002-04-29
Publisher
American Institute of Physics
Citation
Appl. Phys. Lett. 80, 3165 (2002)
Keywords
SOFT PHONON; MODES
Abstract
Effects of the orientation of ferroelectric domains on the characteristics of polarized Raman spectra were studied using an epitaxially grown PbTiO3 thin film in which the c-axis oriented domains coexist with the a-axis oriented domains on MgO (001). To obtain polarized spectra for both two distinctive c and a domains, we have employed scattering configurations in which the relevant phonon wave vector, k, is perpendicular to the c axis of the tetragonal unit cell. Compared with the mode frequencies of single-crystal PbTiO3, a softening of the E(TO) phonons was evident for both c and a domains, suggesting the presence of a strong tensile film stress. In addition to this, we observed a splitting of the degenerate "silent" mode into two distinctive B-1 and E modes in an epitaxially grown film on MgO (001). (C) 2002 American Institute of Physics.
ISSN
0003-6951 (print)1077-3118 (online)
Language
English
URI
http://hdl.handle.net/10371/4904
http://link.aip.org/link/?APPLAB/80/3165/1
DOI
https://doi.org/10.1063/1.1473864
https://doi.org/10.1063/1.1473864
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College of Natural Sciences (자연과학대학)Dept. of Physics and Astronomy (물리·천문학부)Physics (물리학전공)Journal Papers (저널논문_물리학전공)
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