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Charge-Transport Tuning of Solution-Processable Graphene Nanoribbons by Substitutional Nitrogen Doping
Cited 34 time in
Web of Science
Cited 38 time in Scopus
- Authors
- Issue Date
- 2013-12
- Publisher
- John Wiley & Sons Ltd.
- Citation
- Macromolecular Chemistry and Physics, Vol.214 No.23, pp.2768-2773
- Abstract
- Novel nitrogen-doped graphene nanoribbons (GNR-Ns) are synthesized by the coupling reaction between a pyrazine (or benzene) derivative and naphthalene followed by cyclodehydrogenation. The amount of nitrogen doping in the GNR-Ns is controlled by changing the monomer feed ratio of pyrazine to benzene for polymerization. The electron mobility of the GNR-Ns increases while the hole mobility decreases, as the amount of nitrogen doping in the GNR increases, indicating that the charge-transport behavior of GNRs is changed from ambipolar to an n-type semiconductor. The threshold voltage of the GNR-Ns also shifts from 20 to -6 V as the amount of nitrogen doping increases.
- ISSN
- 1022-1352
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