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Catalytic hydrodenitrogenation of indole over molybdenum nitride and carbides with different structures

Cited 81 time in Web of Science Cited 84 time in Scopus
Authors
Li, Sen Zi; Lee, Jae Sung; Hyeon, Taeghwan; Suslick, KS
Issue Date
1999-08
Citation
Applied Catalysis A: General, Vol.184 No.1, pp.1-9
Keywords
hydrodenitrogenationindolemolybdenum nitridemolybdenum carbides
Abstract
The hydrodenitrogenation (HDN) of indole has been studied over Mo2N and Mo2C with different structures. The difference in activity was modest and the structure of the catalysts exerted a more significant effect than the chemical composition. More evident difference was observed in selectivity, and here the composition was the most important factor. Sonochemically prepared Mo2C was an active catalyst for HDN reaction. It formed plate-like aggregates of loosely packed Mo2C (fcc) particles. The crystallinity of sonochemically prepared Mo2C was improved during the reaction, and its behavior in HDN became similar to Mo2C (fcc) prepared by the TPR method. (C) 1999 Elsevier Science B.V. All rights reserved.
ISSN
0926-860X
URI
http://hdl.handle.net/10371/166140
DOI
https://doi.org/10.1016/S0926-860X(99)00044-7
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College of Engineering/Engineering Practice School (공과대학/대학원)Dept. of Chemical and Biological Engineering (화학생물공학부)Journal Papers (저널논문_화학생물공학부)
College of Engineering/Engineering Practice School (공과대학/대학원)Dept. of Chemical and Biological Engineering (화학생물공학부)Chemical Convergence for Energy and Environment (에너지환경 화학융합기술전공)Journal Papers (저널논문_에너지환경 화학융합기술전공)
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