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Electrospun Li-confinable hollow carbon fibers for highly stable Li-metal batteries
DC Field | Value | Language |
---|---|---|
dc.contributor.author | Kim, Byung Gon | - |
dc.contributor.author | Kang, Dong Woo | - |
dc.contributor.author | Park, Gumjae | - |
dc.contributor.author | Park, Sung Hyeon | - |
dc.contributor.author | Lee, Sang -Min | - |
dc.contributor.author | Choi, Jang Wook | - |
dc.date.accessioned | 2022-04-21T00:33:06Z | - |
dc.date.available | 2022-04-21T00:33:06Z | - |
dc.date.created | 2021-07-27 | - |
dc.date.created | 2021-07-27 | - |
dc.date.created | 2021-07-27 | - |
dc.date.created | 2021-07-27 | - |
dc.date.issued | 2021-10-15 | - |
dc.identifier.citation | Chemical Engineering Journal, Vol.422, p. 130017 | - |
dc.identifier.issn | 1385-8947 | - |
dc.identifier.other | 138488 | - |
dc.identifier.uri | https://hdl.handle.net/10371/179163 | - |
dc.description.abstract | Li-metal has steadily gained attention as one of the promising next-generation anode materials because of its exceptional specific capacity and low operating potential that can significantly increase the energy density of batteries beyond those of the state-of-the-art Li-ion batteries. Nevertheless, the use of Li-metal is still faced with the challenge of uncontrollable dendrite growth that ceaselessly causes parasitic reactions, further impeding the practical use of Li-metal batteries. To circumvent this limitation by using a structural approach, herein, we report a 1D hollow carbon fiber incorporating lithiophilic Au nanoparticles (Au@HCF) as a promising Li host that is fabricated by scalable dual-nozzle electrospinning. Due to its well-defined 1D electronic conducting pathways for reducing the effective current density as well as the hollow core for confining Li-metal, Au@HCF can mitigate Li dendrite growth on the top surface and stabilize the solid-electrolyte interphase layer, thereby achieving a high Coulombic efficiency of 99-99.9% under 1 mA cm-2 and 2 mAh cm-2. Moreover, the LiFePO4 full cell combined with the Au@HCF anode containing predeposited 2 mAh cm-2 Li showed considerably improved cycle life of over 380 cycles, indicating that the design concept for the Li-confinable structure can be an excellent option for realizing emerging Li-metal batteries. | - |
dc.language | 영어 | - |
dc.publisher | Elsevier BV | - |
dc.title | Electrospun Li-confinable hollow carbon fibers for highly stable Li-metal batteries | - |
dc.type | Article | - |
dc.contributor.AlternativeAuthor | 최장욱 | - |
dc.identifier.doi | 10.1016/j.cej.2021.130017 | - |
dc.citation.journaltitle | Chemical Engineering Journal | - |
dc.identifier.wosid | 000672587400005 | - |
dc.identifier.scopusid | 2-s2.0-85105254044 | - |
dc.citation.startpage | 130017 | - |
dc.citation.volume | 422 | - |
dc.identifier.sci | 000672587400005 | - |
dc.description.isOpenAccess | N | - |
dc.contributor.affiliatedAuthor | Choi, Jang Wook | - |
dc.type.docType | Article | - |
dc.description.journalClass | 1 | - |
dc.subject.keywordPlus | LITHIUM-METAL | - |
dc.subject.keywordPlus | ANODE | - |
dc.subject.keywordPlus | ELECTROLYTE | - |
dc.subject.keywordPlus | DEPOSITION | - |
dc.subject.keywordPlus | NUCLEATION | - |
dc.subject.keywordPlus | SEPARATORS | - |
dc.subject.keywordPlus | ORIGIN | - |
dc.subject.keywordPlus | MATRIX | - |
dc.subject.keywordPlus | GROWTH | - |
dc.subject.keywordAuthor | Electrospinning | - |
dc.subject.keywordAuthor | Core-shell fiber | - |
dc.subject.keywordAuthor | Lithiophilic material | - |
dc.subject.keywordAuthor | Li host | - |
dc.subject.keywordAuthor | Li-metal battery | - |
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