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Ozone-Treated Carbon Nanotube as a Conductive Agent for Dry-Processed Lithium-Ion Battery Cathode
Cited 6 time in
Web of Science
Cited 6 time in Scopus
- Authors
- Issue Date
- 2023-07
- Publisher
- American Chemical Society
- Citation
- ACS Energy Letters, Vol.8 No.8, pp.3460-3466
- Abstract
- The solvent-free manufacturing process for battery electrodeshasgathered increased scientific interest due to its cost reduction,eco-friendliness, and ability to enhance electrode density. Carbonnanotubes (CNTs) are anticipated to improve battery performance, owingto their exceptional electrical conductivity and unique one-dimensionalmorphology. In this study, we demonstrate that the integration ofozone treatment for CNTs can further enhance the electrochemical performanceof high-loading (30 mg/cm(2) or higher) dry-processed cathodesemploying high-nickel active materials (NCM811). By comparing thesecathodes with dry-processed cathodes using carbon black, a conventionalconductive agent, we elucidate that the enhanced performance of single-walled(SW) CNT-based cathodes originates from the formation of a cathode-electrolyteinterphase with favorable protective abilities and the capacity tosuppress microcrack formation within NCM811 particles. The currentstudy presents a promising strategy of incorporating SWCNTs with thetuned surface functionalities for the development of cost-effective,environmentally friendly dry battery manufacturing.
- ISSN
- 2380-8195
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