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Preventing hydrates cohesion with a bio-inspired vitamin E derivative
Cited 6 time in
Web of Science
Cited 5 time in Scopus
- Authors
- Issue Date
- 2019-12-01
- Publisher
- Elsevier BV
- Citation
- Fuel, Vol.257, p. 116035
- Abstract
- A solidified natural gas (SNG) technology was investigated to transport natural gas in a hydrate slurry. A Vitamin E derivative (D-alpha tocopherol succinate, Vitamin E-TS), which is naturally derived and readily available, was used to disperse water in the decane phase under the turbulent mixing condition. Compared to other non-ionic or cationic surfactants, Vitamin E-TS induced fast hydrate formation and a high conversion rate with an advantage of maintaining flowability during hydrate formation. For example, when using sorbitan monostearate (Span-60), hydrates grew to form a thick layer at the decane/water interface. Due to the strong cohesion of hydrate in the layer, a high relative torque was observed on mixing and the impeller was stopped. Moreover, dodecyl-trimethylammonium bromide (DTAB) showed increased relative torque in the early stage of hydrate formation. From the experimental results under both steady and dynamic operating conditions, Vitamin E-TS showed the optimal performance in quickly producing hydrate slurries and high conversion while maintaining fluid flowability. Accordingly, a continuous process was proposed to use water and decane as feed to produce the hydrate slurry in the presence of Vitamin E-TS.
- ISSN
- 0016-2361
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