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Proton irradiation effects on mechanochemically synthesized and flash-evaporated hybrid organic-inorganic lead halide perovskites

Cited 1 time in Web of Science Cited 2 time in Scopus
Authors

Shin, Jiwon; Baek, Kyeong-Yoon; Lee, Jonghoon; Lee, Woocheol; Kim, Jaeyoung; Jang, Juntae; Park, Jaehyoung; Kang, Keehoon; Cho, Kyungjune; Lee, Takhee

Issue Date
2022-02
Publisher
Institute of Physics Publishing
Citation
Nanotechnology, Vol.33 No.6, p. 065706
Abstract
A hybrid organic-inorganic halide perovskite is a promising material for developing efficient solar cell devices, with potential applications in space science. In this study, we synthesized methylammonium lead iodide (MAPbI(3)) perovskites via two methods: mechanochemical synthesis and flash evaporation. We irradiated these perovskites with highly energetic 10 MeV proton-beam doses of 10(11), 10(12), 10(13), and 4 x 10(13) protons cm(-2) and examined the proton irradiation effects on the physical properties of MAPbI(3) perovskites. The physical properties of the mechanochemically synthesized MAPbI(3) perovskites were not considerably affected after proton irradiation. However, the flash-evaporated MAPbI(3) perovskites showed a new peak in x-ray diffraction and an increased fluorescence lifetime in time-resolved photoluminescence under high-dose conditions, indicating considerable changes in their physical properties. This difference in behavior between MAPbI(3) perovskites synthesized via the abovementioned two methods may be attributed to differences in radiation hardness associated with the bonding strength of the constituents, particularly Pb-I bonds. Our study will help to understand the radiation effect of proton beams on organometallic halide perovskite materials.
ISSN
0957-4484
URI
https://hdl.handle.net/10371/202514
DOI
https://doi.org/10.1088/1361-6528/ac34a7
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  • College of Engineering
  • Department of Materials Science & Engineering
Research Area Molecular doping in emerging semiconductors, Next-generation electronic devices, Transport phenomena in organic semiconductors

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