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Recent Progress in High Donor Electrolytes for Lithium-Sulfur Batteries
DC Field | Value | Language |
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dc.contributor.author | Shin, Hyuksoo | - |
dc.contributor.author | Baek, Minsung | - |
dc.contributor.author | Gupta, Abhay | - |
dc.contributor.author | Char, Kookheon | - |
dc.contributor.author | Manthiram, Arumugam | - |
dc.contributor.author | Choi, Jang Wook | - |
dc.date.accessioned | 2023-03-24T01:05:13Z | - |
dc.date.available | 2023-03-24T01:05:13Z | - |
dc.date.created | 2021-02-01 | - |
dc.date.created | 2021-02-01 | - |
dc.date.created | 2021-02-01 | - |
dc.date.created | 2021-02-01 | - |
dc.date.issued | 2020-07 | - |
dc.identifier.citation | Advanced Energy Materials, Vol.10 No.27, p. 2001456 | - |
dc.identifier.issn | 1614-6832 | - |
dc.identifier.uri | https://hdl.handle.net/10371/189740 | - |
dc.description.abstract | Lithium-sulfur (Li-S) batteries continue to be considered promising post-lithium-ion batteries owing to their high theoretical energy density. In pursuit of a Li-S cell with long-term cyclability, most studies thus far have relied on using ether-based electrolytes. However, their limited ability to dissolve polysulfides requires a high electrolyte-to-sulfur ratio, which impairs the achievable specific energy. Recently, the battery community found high donor electrolytes to be a potential solution to this shortcoming because their high solubility toward polysulfides enables a cell to operate under lean electrolyte conditions. Despite the increasing number of promising outcomes with high donor electrolytes, a critical hurdle related to stability of the lithium-metal counter electrode needs to be overcome. This review provides an overview of recent efforts pertaining to high donor electrolytes in Li-S batteries and is intended to raise interest from within the community. Furthermore, based on analogous efforts in the lithium-air battery field, strategies for protecting the lithium metal electrode are proposed. It is predicted that high donor electrolytes will be elevated to a higher status in the field of Li-S batteries, with the hope that either existing or upcoming strategies will, to a fair extent, mitigate the degradation of the lithium-metal interface. | - |
dc.language | 영어 | - |
dc.publisher | Wiley-VCH Verlag | - |
dc.title | Recent Progress in High Donor Electrolytes for Lithium-Sulfur Batteries | - |
dc.type | Article | - |
dc.identifier.doi | 10.1002/aenm.202001456 | - |
dc.citation.journaltitle | Advanced Energy Materials | - |
dc.identifier.wosid | 000535816700001 | - |
dc.identifier.scopusid | 2-s2.0-85085623779 | - |
dc.citation.number | 27 | - |
dc.citation.startpage | 2001456 | - |
dc.citation.volume | 10 | - |
dc.description.isOpenAccess | Y | - |
dc.contributor.affiliatedAuthor | Char, Kookheon | - |
dc.contributor.affiliatedAuthor | Choi, Jang Wook | - |
dc.type.docType | Review | - |
dc.description.journalClass | 1 | - |
dc.subject.keywordPlus | DIMETHYLSULFOXIDE-BASED ELECTROLYTE | - |
dc.subject.keywordPlus | IN-SALT ELECTROLYTE | - |
dc.subject.keywordPlus | LI-ION BATTERIES | - |
dc.subject.keywordPlus | LONG-CYCLE-LIFE | - |
dc.subject.keywordPlus | METAL ANODE | - |
dc.subject.keywordPlus | LI-O-2 BATTERY | - |
dc.subject.keywordPlus | POROUS CARBON | - |
dc.subject.keywordPlus | ELECTROCHEMICAL REDUCTION | - |
dc.subject.keywordPlus | POLYSULFIDE MEDIATOR | - |
dc.subject.keywordPlus | DENDRITIC GROWTH | - |
dc.subject.keywordAuthor | disproportionation | - |
dc.subject.keywordAuthor | high donor electrolytes | - |
dc.subject.keywordAuthor | lithium-metal anodes | - |
dc.subject.keywordAuthor | lithium-sulfur batteries | - |
dc.subject.keywordAuthor | polysulfides | - |
dc.subject.keywordAuthor | shuttling effects | - |
dc.subject.keywordAuthor | sulfur radical | - |
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