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Translating the Optimized Durability of Co-Based Anode Catalyst into Sustainable Anion Exchange Membrane Water Electrolysis

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dc.contributor.authorHan, Sanghwi-
dc.contributor.authorRyu, Jae Hyun-
dc.contributor.authorLee, Won Bo-
dc.contributor.authorRyu, Jaeyune-
dc.contributor.authorYoon, Jeyong-
dc.date.accessioned2024-05-17T07:35:45Z-
dc.date.available2024-05-17T07:35:45Z-
dc.date.created2024-04-08-
dc.date.issuedACCEPT-
dc.identifier.citationSmall-
dc.identifier.issn1613-6810-
dc.identifier.urihttps://hdl.handle.net/10371/203138-
dc.description.abstractDevelopment of robust electrocatalysts for the oxygen evolution reaction (OER) underpins the efficient production of green hydrogen via anion exchange membrane water electrolysis (AEMWE). This study elucidates the factors contributing to the degradation of cobalt-based (Co-based) OER catalysts synthesized via electrodeposition, thus establishing strategic approaches to enhance their longevity. Systematic variations in the electroplating process and subsequent heat treatment reveal a delicate balance between catalytic activity and durability, substantiated by comprehensive electrochemical assessments and material analyses. Building upon these findings, the Co-based anode is successfully optimized in the AEMWE single-cell configuration, showcasing an average degradation rate of 0.07 mV h-1 over a continuous operation for 1500 h at a current density of 1 A cm-2. An efficient strategy for enhancing the durability of Co-based oxygen evolution catalyst is proposed. Through meticulous control of the electroplating and subsequent heat treatment, the durability is successfully improved at the expense of the initial performance. The optimized anode demonstrates exceptional durability for 1500 h at a current density of 1 A cm-2 in an anion exchange water electrolysis single-cell. image-
dc.language영어-
dc.publisherWiley - V C H Verlag GmbbH & Co.-
dc.titleTranslating the Optimized Durability of Co-Based Anode Catalyst into Sustainable Anion Exchange Membrane Water Electrolysis-
dc.typeArticle-
dc.identifier.doi10.1002/smll.202311052-
dc.citation.journaltitleSmall-
dc.identifier.wosid001150641300001-
dc.identifier.scopusid2-s2.0-85183360943-
dc.description.isOpenAccessN-
dc.contributor.affiliatedAuthorRyu, Jaeyune-
dc.contributor.affiliatedAuthorYoon, Jeyong-
dc.type.docTypeArticle; Early Access-
dc.description.journalClass1-
dc.subject.keywordPlusOXYGEN EVOLUTION REACTION-
dc.subject.keywordPlusPERFORMANCE-
dc.subject.keywordPlusRECONSTRUCTION-
dc.subject.keywordPlusSTABILITY-
dc.subject.keywordPlusCOOOH-
dc.subject.keywordAuthoranion exchange membrane water electrolysis-
dc.subject.keywordAuthorcobalt-
dc.subject.keywordAuthordurability-
dc.subject.keywordAuthorelectrocatalysts-
dc.subject.keywordAuthoroxygen vacancy-
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  • College of Engineering
  • School of Chemical and Biological Engineering
Research Area Catalysis, Nano Materials, Physical E-Chem, 무기화학, 물리전기화학

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