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Development of a multi-layered micro-reactor coated with Pt–Co/Al2O3 catalyst for preferential oxidation of CO

Cited 19 time in Web of Science Cited 19 time in Scopus
Authors
Kim, Kyung-Yeol; Nam, Suk-Woo; Han, Jonghee; Yoon, Sung Pil; Lim, Tae-Hoon; Lee, Ho-In
Issue Date
2008
Publisher
Elsevier
Citation
Journal of Industrial and Engineering Chemistry 14 (2008) 853–859
Keywords
Preferential oxidationPt–Co/Al2O3Micro-reactorFuel processor
Abstract
Pt–Co/Al2O3 catalysts were prepared with different Co/Pt weight ratios (0.3–1.8) and their performances for preferential oxidation of CO
(PROX) were tested. The activity of the catalyst increased with Co/Pt weight ratio due to the increase of the area of active phase by interaction
between Pt and Co species. The 13-layered micro-channel reactor was prepared by stacking the plates coated with Pt–Co/Al2O3 catalyst. The
reactor was divided into three parts (inlet, middle, and outlet) to evaluate the performance of each part. Most of O2 supplied was depleted at the inlet
part and the temperature gradient of the reactor occurred due to the high exothermicity of oxidations of CO and hydrogen. In order to prevent hot
spot and temperature gradient, the reactor with non-uniform distribution of the catalyst (partially coating the catalyst on the channels) was
prepared. The prepared reactor showed uniform temperature distribution and exhibited excellent performance for PROX.
ISSN
1226-086X
Language
English
URI
https://hdl.handle.net/10371/61321
DOI
https://doi.org/10.1016/j.jiec.2008.05.003
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College of Engineering/Engineering Practice School (공과대학/대학원)Dept. of Chemical and Biological Engineering (화학생물공학부)Journal Papers (저널논문_화학생물공학부)
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